Photon Statistics for Single Molecule Non-Linear Spectroscopy

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dc.creatorShikerman, F.
dc.creatorBarkai, E.
dc.date2007-05-28
dc.date.accessioned2026-07-07T08:53:44Z
dc.date.available2026-07-07T08:53:44Z
dc.descriptionWe consider the theory of the non-linear spectroscopy for a single molecule undergoing stochastic dynamics and interacting with a sequence of two laser pulses. General expressions for photon counting statistics are obtained, and an exact solution to the problem of the Kubo-Anderson process is found. In the limit of impulsive pulses the information on the photon statistics is contained in the molecule's dipole correlation function. The selective limit where temporal resolution is maintained, the semi-classical approximation and the fast modulation limit exhibit general behaviors of this new type of spectroscopy. We show how the design of the external field leads to rich insights on dynamics of individual molecules which are different than those found for an ensemble.
dc.identifierhttps://arxiv.org/abs/0705.4028
dc.identifierhttp://arxiv.org/abs/0705.4028
dc.identifierPhys. Rev. Lett. 99, 208302 (2007)
dc.identifierdoi:10.1103/PhysRevLett.99.208302
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/145726
dc.subjectOptics
dc.subjectChemical Physics
dc.titlePhoton Statistics for Single Molecule Non-Linear Spectroscopy
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