Two-Photon Emission from Semiconductors
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We report the first experimental observations of two-photon emission from semiconductors, to the best of our knowledge, and develop a corresponding theory for the room-temperature process. Spontaneous two-photon emission is demonstrated in optically-pumped bulk GaAs and in electrically-driven GaInP/AlGaInP quantum wells. Singly-stimulated two-photon emission measurements demonstrate the theoretically predicted two-photon optical gain in semiconductors - a necessary ingredient for any realizations of future two-photon semiconductor lasers. Photon-coincidence experiment validates the simultaneity of the electrically-driven GaInP/AlGaInP two-photon emission, limited only by detector's temporal resolution.
Coincidence experiment results added, QW stimulated TPE added, stimulation power TPE dependence shown, measured spectra recalibrated, quantitative theory presented
Coincidence experiment results added, QW stimulated TPE added, stimulation power TPE dependence shown, measured spectra recalibrated, quantitative theory presented