Dynamical symmetry breaking in transport through molecules

dc.creatorDonarini, Andrea
dc.creatorGrifoni, Milena
dc.creatorRichter, Klaus
dc.date2006-05-04
dc.date2006-10-17
dc.date.accessioned2026-07-07T07:08:45Z
dc.date.available2026-07-07T07:08:45Z
dc.descriptionWe analyze the interplay between vibrational and electronic degrees of freedom in charge transport across a molecular single-electron transistor. We focus on the wide class of molecules which possess quasi-degenerate vibrational eigenstates, while no degeneracy occurs for their anionic configuration. We show that the combined effect of a thermal environment and coupling to leads, involving tunneling events charging and discharging the molecule, leads to a dynamical symmetry breaking where quasi-degenerate eigenstates acquire different occupations. This imbalance gives rise to a characteristic asymmetry of the current versus an applied gate voltage.
dc.description4 pages, 2 figures, revised final published version
dc.identifierhttps://arxiv.org/abs/cond-mat/0605123
dc.identifierhttp://arxiv.org/abs/cond-mat/0605123
dc.identifierPhys. Rev. Lett. 97, 166801 (2006)
dc.identifierdoi:10.1103/PhysRevLett.97.166801
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/110823
dc.subjectSoft Condensed Matter
dc.titleDynamical symmetry breaking in transport through molecules
dc.typetext

Files

Collections