Ab initio phonon dispersion curves and interatomic force constants of barium titanate

dc.creatorGhosez, Ph.
dc.creatorGonze, X.
dc.creatorMichenaud, J. -P.
dc.date1997-06-30
dc.date.accessioned2026-07-07T09:11:52Z
dc.date.available2026-07-07T09:11:52Z
dc.descriptionThe phonon dispersion curves of cubic BaTiO_3 have been computed within a first-principles approach and the results compared to the experimental data. The curves obtained are very similar to those reported for KNbO_3 by Yu and Krakauer [Phys. Rev. Lett. 74, 4067 (1995)]. They reveal that correlated atomic displacements along <100> chains are at the origin of the ferroelectric instability. A simplified model illustrates that spontaneous collective displacements will occur when a dozen of aligned atoms are coupled. The longitudinal interatomic force constant between nearest neighbour Ti and O atoms is relatively weak in comparison to that between Ti atoms in adjacent cells. The small coupling between Ti and O displacements seems however necessary to reproduce a ferroelectric instability.
dc.description12 pages, 4 figures
dc.identifierhttps://arxiv.org/abs/cond-mat/9706294
dc.identifierhttp://arxiv.org/abs/cond-mat/9706294
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/151835
dc.subjectMaterials Science
dc.titleAb initio phonon dispersion curves and interatomic force constants of barium titanate
dc.typetext

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