Sticky obstacles to intramolecular energy flow

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dc.creatorPaškauskas, R.
dc.creatorChandre, C.
dc.creatorUzer, T.
dc.date2007-08-14
dc.date.accessioned2026-07-07T13:10:15Z
dc.date.available2026-07-07T13:10:15Z
dc.descriptionVibrational energy flows unevenly in molecules, repeatedly going back and forth between trapping and roaming. We identify bottlenecks between diffusive and chaotic behavior, and describe generic mechanisms of these transitions, taking the carbonyl sulphide molecule OCS as a case study. The bottlenecks are found to be lower-dimensional tori; their bifurcations and unstable manifolds govern the transition mechanisms.
dc.description4 pages, 4 figures
dc.identifierhttps://arxiv.org/abs/0708.1893
dc.identifierhttp://arxiv.org/abs/0708.1893
dc.identifierPhysical Review Letters 100, 083001 (2008)
dc.identifierdoi:10.1103/PhysRevLett.100.083001
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/228962
dc.subjectChaotic Dynamics
dc.subjectChemical Physics
dc.titleSticky obstacles to intramolecular energy flow
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