Systematic Perturbation Theory for Dynamical Coarse-Graining
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We demonstrate how the dynamical coarse-graining approach can be systematically extended to higher orders in the coupling between system and reservoir. Up to second order in the coupling constant we explicitly show that dynamical coarse-graining unconditionally preserves positivity of the density matrix -- even for bath density matrices that are not in equilibrium and also for time-dependent system Hamiltonians. By construction, the approach correctly captures the short-time dynamics, i.e., it is suitable to analyze non-Markovian effects. We compare the dynamics with the exact solution for highly non-Markovian systems and find a remarkable quality of the coarse-graining approach. The extension to higher orders is straightforward but rather tedious. The approach is especially useful for bath correlation functions of simple structure and for small system dimensions.
17 pages, 5 figures, version accepted for publication in PRA
17 pages, 5 figures, version accepted for publication in PRA