Photoemission study of polycrystalline Gd_{1-x}Sr_xTiO_{3+delta}: correlation and surface effects

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dc.creatorSing, M.
dc.creatorKarlsson, M.
dc.creatorSchrupp, D.
dc.creatorClaessen, R.
dc.creatorHeinrich, M.
dc.creatorFritsch, V.
dc.creatorvon Nidda, H. -A. Krug
dc.creatorLoidl, A.
dc.creatorBulla, R.
dc.date2002-05-03
dc.date.accessioned2026-07-07T02:45:18Z
dc.date.available2026-07-07T02:45:18Z
dc.descriptionWe report photoemission studies of polycrystalline samples of Sr-doped GdTiO_{3+delta}, which undergoes a Mott-Hubbard-like metal-insulator transition at a Ti-concentration of about 20%. The Ti 3d-derived valence band near the Fermi level displays a two-peak structure consistent with a Hubbard-model-type interpretation as quasiparticle and lower Hubbard band. Contrary to the theoretical expectation the lower Hubbard band does not change its energy with doping. However, the analysis of the core level spectra and elemental mapping with a scanning electron microscope indicate a strongly inhomogeneous doping concentration in the probed surface regions. This questions the intrinsic character of the valence band spectra and demonstrates a general difficulty when using polycrystalline samples for such studies.
dc.identifierhttps://arxiv.org/abs/cond-mat/0205067
dc.identifierhttp://arxiv.org/abs/cond-mat/0205067
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/19251
dc.subjectStrongly Correlated Electrons
dc.titlePhotoemission study of polycrystalline Gd_{1-x}Sr_xTiO_{3+delta}: correlation and surface effects
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