A New Type of Two-photon Forward Radiation in Pure Liquids

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Unexpected spectral features are observed in the two photon spectrum of the pure water in the forward direction when an 80 femtosecond laser pulse is focused at 10^10Wcm-2 or less. Such intensity is much lower than the breakdown or stimulated threshold of the liquid water. The two broad features are about 2700cm-1 and 5000cm-1 red shifted from the hyper-Rayleigh wavelength, respectively, and they are quadratic with the laser intensity. They do not match the known Raman or hyper-Raman frequencies of water, and they are both centered at a narrow angle in the forward direction. Several other liquids also exhibited similar but molecular specific spectral features.
4 pages, 4 figures

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Chemical Physics, Optics

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http://salesiana.dossiersoluciones.com/handle/123456789/131883

Consulte el texto completo en el siguiente enlace:

https://arxiv.org/abs/0706.2408
 http://arxiv.org/abs/0706.2408

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arXiv