Photon-correlation Fourier spectroscopy

dc.creatorBrokmann, Xavier
dc.creatorBawendi, Moungi
dc.creatorCoolen, Laurent
dc.creatorhermier, Jean-Pierre
dc.date2006-04-21
dc.date.accessioned2026-07-07T12:52:01Z
dc.date.available2026-07-07T12:52:01Z
dc.descriptionWe describe a method to probe the spectral fluctuations of a transition over broad ranges of frequencies and timescales with the high spectral resolution of Fourier spectroscopy, and a temporal resolution as high as the excited state lifetime, even in the limit of very low photocounting rates. The method derives from a simple relation between the fluorescence spectral dynamics of a single radiating dipole and its fluorescence intensity correlations at the outputs of a continuously scanning Michelson interferometer. These findings define an approach to investigate the fast fluorescence spectral dynamics of single molecules and other faint light sources beyond the time-resolution capabilities of standard spectroscopy experiments.
dc.description7 pages, 3 figures
dc.identifierhttps://arxiv.org/abs/physics/0604180
dc.identifierhttp://arxiv.org/abs/physics/0604180
dc.identifierOptics Express, Vol. 14, Issue 13, pp. 6333-6341 (2006)
dc.identifierdoi:10.1364/OE.14.006333
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/223169
dc.subjectOptics
dc.titlePhoton-correlation Fourier spectroscopy
dc.typetext

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