Photo-induced intermolecular charge transfer in porphyrin complexes

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dc.creatorSchreiber, Michael
dc.creatorKilin, Dmitry
dc.creatorKleinekathoefer, Ulrich
dc.date2000-01-06
dc.date.accessioned2026-07-07T05:43:33Z
dc.date.available2026-07-07T05:43:33Z
dc.descriptionOptical excitation of the sequential supermolecule H_2P-ZnP-Q induces an electron transfer from the free-base porphyrin (H_2P) to the quinone (Q) via the zinc porphyrin (ZnP). This process is modeled by equations of motion for the reduced density matrix which are solved numerically and approximately analytically. These two solutions agree very well in a great region of parameter space. It is shown that for the majority of solvents the electron transfer occurs with the superexchange mechanism.
dc.descriptionThe deep analysis of this problem has been presented in Ph. D. thesis http://xxx.lanl.gov/abs/quant-ph/0001004
dc.identifierhttps://arxiv.org/abs/physics/0001014
dc.identifierhttp://arxiv.org/abs/physics/0001014
dc.identifierExciton Processes in Condensed Matter, Editors: R. T. Williams and W. H. Yen, PV98-25, (The Electrochemical Society Proceedings Series, Pennington, NJ 1998), p. 99
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/83346
dc.subjectChemical Physics
dc.subjectBiological Physics
dc.titlePhoto-induced intermolecular charge transfer in porphyrin complexes
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