Spectrally Narrowed Edge Emission from Organic Light-Emitting Diodes: Evidence for Amplified Spontaneous Emission and Mirrorless Lasing

dc.creatorTian, Yun
dc.creatorGan, Zhengqing
dc.creatorZhou, Zhaoqun
dc.creatorKang, Ji-hun
dc.creatorPark, Q-Han
dc.creatorLynch, David W.
dc.creatorShinar, Joseph
dc.date2007-01-14
dc.date.accessioned2026-07-07T07:40:51Z
dc.date.available2026-07-07T07:40:51Z
dc.descriptionp-Conjugated materials, including small molecules and polymers, are attracting substantial attention as novel gain media in semiconductor lasers; they offer many potential advantages not achievable with conventional inorganic semiconductors: simple processing, low cost, easy tuneability of the spectrum, and large-area integration on flexible substrates. Optically pumped lasing action in various small molecular and polymeric p-conjugated materials has been demonstrated using several resonator configurations. However, electrically pumped organic semiconductor lasers, i.e., organic injection or diode lasers, remain elusive, presumably due to various loss mechanisms, e.g., charge (polaron)-induced absorption and metal electrode absorption. Here we report on evidence for amplified spontaneous emission (ASE), also known as mirrorless lasing (i.e., wherein some of the spontaneously emitted photons are amplified by stimulated emission during their propagation) in DC-driven small molecular organic light-emitting diodes (SMOLEDs). The evidence includes a dramatic spectral line narrowing, with a full width at half maximum (FWHM) of only 5 - 10 nm, and optical gain, of the edge-emission from SMOLEDs at room temperature. However, there is no clear indication of threshold behavior associated with this spectral narrowing. Nevertheless, this discovery should pave the way towards the realization of an organic diode laser.
dc.description14 pages, 5 figures
dc.identifierhttps://arxiv.org/abs/cond-mat/0701312
dc.identifierhttp://arxiv.org/abs/cond-mat/0701312
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/121904
dc.subjectMaterials Science
dc.subjectSoft Condensed Matter
dc.titleSpectrally Narrowed Edge Emission from Organic Light-Emitting Diodes: Evidence for Amplified Spontaneous Emission and Mirrorless Lasing
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