Orbital Dependent Exchange-Only Methods for Periodic Systems

dc.creatorS"ule, P.
dc.creatorKurth, S.
dc.creatorVan Doren, V.
dc.date1999-07-19
dc.date.accessioned2026-07-07T03:13:56Z
dc.date.available2026-07-07T03:13:56Z
dc.descriptionVarious orbital-dependent exchange-only potentials are studied which exhibit correct long-range asymptotic behaviour. We present the first application of these potentials for polymers and by one of these potentials for molecules. Kohn-Sham type calculations have been carried out for polyethylene in order to make valuable comparison of these potentials with each other as well as with Hartree-Fock and exchange-only LDA methods. The Kohn-Sham band gap obtained with the optimized effective potetial method is corrected with the exchange contribution to the derivative discontinuity of the exchange-correlation potential. The corrected band gap obtained with the Slater's exchange potential is 9.7 eV close to the experiment.
dc.description11 pages, 2 figures. Phys. Rev. B60, 1999, in press
dc.identifierhttps://arxiv.org/abs/cond-mat/9907274
dc.identifierhttp://arxiv.org/abs/cond-mat/9907274
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/29495
dc.subjectCondensed Matter
dc.titleOrbital Dependent Exchange-Only Methods for Periodic Systems
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