LaCoO3 - from first principles

dc.creatorRadwanski, R. J.
dc.creatorRopka, Z.
dc.date2006-03-23
dc.date.accessioned2026-07-07T07:04:54Z
dc.date.available2026-07-07T07:04:54Z
dc.descriptionWe have performed calculations of the electronic structure of LaCoO3 from first principles, assuming the atomistic construction of matter and the electrostatic origin of the crystal-field splitting. In our atomic-like approach QUASST the d electrons of the Co3+ ion in LaCoO3 form the highly-correlated atomic-like system 3d6 with the singlet ground state 1A1 (an octahedral subterm from the 1I term) and the excited octahedral subterm 5T2g of the 5D term. In the spin-orbital space, being physically adequate, this high-spin state is Jahn-Teller active. We take the ESR experiment of Noguchi et al., Phys. Rev. B 66, 094404 (2002), as confirmation of the existence of the discrete electronic structure for 3$d$ electron states in LaCoO3 in the meV scale postulated in QUASST.
dc.description4 pages, 1 figure embedded
dc.identifierhttps://arxiv.org/abs/cond-mat/0603619
dc.identifierhttp://arxiv.org/abs/cond-mat/0603619
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/109490
dc.subjectStrongly Correlated Electrons
dc.titleLaCoO3 - from first principles
dc.typetext

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