Overlapping resonances in the control of intramolecular vibrational redistribution

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Coherent control of bound state processes via the interfering overlapping resonances scenario [Christopher et al., J. Chem. Phys. 123, 064313 (2006)] is developed to control intramolecular vibrational redistribution (IVR). The approach is applied to the flow of population between bonds in a model of chaotic OCS vibrational dynamics, showing the ability to significantly alter the extent and rate of IVR by varying quantum interference contributions.
10 pages, 7 figures

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Quantum Physics

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http://salesiana.dossiersoluciones.com/handle/123456789/126550

Consulte el texto completo en el siguiente enlace:

https://arxiv.org/abs/quant-ph/0703263
 http://arxiv.org/abs/quant-ph/0703263
 J. Chem. Phys. 126, 124307 (2007)
 doi:10.1063/1.2710791

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arXiv