Driven polymer translocation through a nanopore: a manifestation of anomalous diffusion

dc.creatorDubbeldam, J. L. A.
dc.creatorMilchev, A.
dc.creatorRostiashvili, V. G.
dc.creatorVilgis, T. A.
dc.date2007-02-20
dc.date2007-06-05
dc.date.accessioned2026-07-07T08:20:37Z
dc.date.available2026-07-07T08:20:37Z
dc.descriptionWe study the translocation dynamics of a polymer chain threaded through a nanopore by an external force. By means of diverse methods (scaling arguments, fractional calculus and Monte Carlo simulation) we show that the relevant dynamic variable, the translocated number of segments $s(t)$, displays an {\em anomalous} diffusive behavior even in the {\em presence} of an external force. The anomalous dynamics of the translocation process is governed by the same universal exponent $α= 2/(2ν+2 - γ_1)$, where $ν$ is the Flory exponent and $γ_1$ - the surface exponent, which was established recently for the case of non-driven polymer chain threading through a nanopore. A closed analytic expression for the probability distribution function $W(s, t)$, which follows from the relevant {\em fractional} Fokker - Planck equation, is derived in terms of the polymer chain length $N$ and the applied drag force $f$. It is found that the average translocation time scales as $τ\propto f^{-1}N^{\frac{2}α -1}$. Also the corresponding time dependent statistical moments, $< s(t) > \propto t^α$ and $< s(t)^2 > \propto t^{2α}$ reveal unambiguously the anomalous nature of the translocation dynamics and permit direct measurement of $α$ in experiments. These findings are tested and found to be in perfect agreement with extensive Monte Carlo (MC) simulations.
dc.description6 pages, 4 figures, accepted to Europhys. Lett; some references were supplemented; typos were corrected
dc.identifierhttps://arxiv.org/abs/cond-mat/0702463
dc.identifierhttp://arxiv.org/abs/cond-mat/0702463
dc.identifierEurophys. Lett. 79, 18002 (2007)
dc.identifierdoi:10.1209/0295-5075/79/18002
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/135121
dc.subjectStatistical Mechanics
dc.subjectSoft Condensed Matter
dc.titleDriven polymer translocation through a nanopore: a manifestation of anomalous diffusion
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