Chain Diffusion in Lamellar Block Copolymers

dc.creatorMurat, Michael
dc.creatorGrest, Gary S.
dc.creatorKremer, Kurt
dc.date1997-05-28
dc.date.accessioned2026-07-07T09:11:48Z
dc.date.available2026-07-07T09:11:48Z
dc.descriptionDiffusion of symmetric diblock copolymer chains in macroscopically oriented lamellar block copolymers are studied in a molecular dynamics simulation. Results for diffusion constant both parallel $D_\parallel$ and perpendicular $D_\perp$ to the lamellar planes are compared to results in the disordered one phase region. For diblocks of length N=40 (1.1 N_e) and $100 (3N_e)$, where $N_e$ is the entanglement length of a homopolymer melt at the same density, $D_\parallel$ is nearly independent of $χ$, while $D_\perp$ is strongly suppressed as $χ$ is increased. These results are in agreement with theoretical predictions based on the Rouse model. The isotropic diffusion constant of quenched disordered systems is approximated fairly well by $(2D_\parallel+D_\perp)/3$ of the corresponding lamellar system.
dc.descriptionRevtex 12 pages, 4 postscript figures, uses psfig
dc.identifierhttps://arxiv.org/abs/cond-mat/9705293
dc.identifierhttp://arxiv.org/abs/cond-mat/9705293
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/151807
dc.subjectSoft Condensed Matter
dc.subjectMaterials Science
dc.titleChain Diffusion in Lamellar Block Copolymers
dc.typetext

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