Nonlinear optical response in higher fullerenes

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Nonlinear optical properties of extracted higher fullerenes - C70, C76, C78, and C84 - are theoretically investigated. Magnitudes of off-resonant third-harmonic-generation are calculated by the intermediate exciton theory. We find that optical nonlinearities of higher fullerenes are a few times larger than those of C60. The magnitudes of nonlinearity tend to increase as the optical gap decreases in higher fullerenes.
Condensed Matter Theory Group at ETL: http://www.etl.go.jp/Organization/Bussei-kiso/

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Condensed Matter, Chemical Physics, Optics

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http://salesiana.dossiersoluciones.com/handle/123456789/151718

Consulte el texto completo en el siguiente enlace:

https://arxiv.org/abs/cond-mat/9702181
 http://arxiv.org/abs/cond-mat/9702181
 Jpn. J. Appl. Phys. 36 (1997) L485-L487
 doi:10.1143/JJAP.36.L485

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arXiv