Polymer Translocation out of Planar Confinements

dc.creatorPanja, Debabrata
dc.creatorBarkema, Gerard T.
dc.creatorBall, Robin C.
dc.date2007-09-30
dc.date2007-11-19
dc.date.accessioned2026-07-07T08:56:39Z
dc.date.available2026-07-07T08:56:39Z
dc.descriptionPolymer translocation in three dimensions out of planar confinements is studied in this paper. Three membranes are located at $z=-h$, $z=0$ and $z=h_1$. These membranes are impenetrable, except for the middle one at $z=0$, which has a narrow pore. A polymer with length $N$ is initially sandwiched between the membranes placed at $z=-h$ and $z=0$ and translocates through this pore. We consider strong confinement (small $h$), where the polymer is essentially reduced to a two-dimensional polymer, with a radius of gyration scaling as $R^{\tinytext{(2D)}}_g \sim N^{ν_{\tinytext{2D}}}$; here, $ν_{\tinytext{2D}}=0.75$ is the Flory exponent in two dimensions. The polymer performs Rouse dynamics. Based on theoretical analysis and high-precision simulation data, we show that in the unbiased case $h=h_1$, the dwell-time $τ_d$ scales as $N^{2+ν_{\tinytext{2D}}}$, in perfect agreement with our previously published theoretical framework. For $h_1=\infty$, the situation is equivalent to field-driven translocation in two dimensions. We show that in this case $τ_d$ scales as $N^{2ν_{\tinytext{2D}}}$, in agreement with several existing numerical results in the literature. This result violates the earlier reported lower bound $N^{1+ν}$ for $τ_d$ for field-driven translocation. We argue, based on energy conservation, that the actual lower bound for $τ_d$ is $N^{2ν}$ and not $N^{1+ν}$. Polymer translocation in such theoretically motivated geometries thus resolves some of the most fundamental issues that are the subjects of much heated debate in recent times.
dc.descriptionMinor changes; 18+ pages, 8 figures, 5 tables, to appear in J. Phys: Cond. Mat
dc.identifierhttps://arxiv.org/abs/0710.0147
dc.identifierhttp://arxiv.org/abs/0710.0147
dc.identifierJ. Phys.: Condens. Matter 20, 075101 (2008)
dc.identifierdoi:10.1088/0953-8984/20/7/075101
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/146685
dc.subjectSoft Condensed Matter
dc.subjectStatistical Mechanics
dc.titlePolymer Translocation out of Planar Confinements
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