Solution of the crystallographic phase problem by iterated projections

dc.creatorElser, Veit
dc.date2002-09-30
dc.date.accessioned2026-07-07T02:47:31Z
dc.date.available2026-07-07T02:47:31Z
dc.descriptionAn algorithm for determining crystal structures from diffraction data is described which does not rely on the usual Fourier-space formulations of atomicity. The new algorithm implements atomicity constraints in real-space, as well as intensity constraints in Fourier-space, by projections which restore each constraint with the minimal modification of the scattering density. To recover the true density, the two projections are combined into a single operation, the difference map, which is iterated until the magnitude of the density modification becomes acceptably small. The resulting density, when acted upon by a single additional operation, is by construction a density which satisfies both intensity and atomicity constraints. Numerical experiments have yielded solutions for atomic resolution x-ray data sets with over 400 non-hydrogen atoms, as well as for neutron data, where positivity of the density cannot be invoked.
dc.description14 pages, 9 figures
dc.identifierhttps://arxiv.org/abs/cond-mat/0209690
dc.identifierhttp://arxiv.org/abs/cond-mat/0209690
dc.identifier.urihttp://salesiana.dossiersoluciones.com/handle/123456789/20036
dc.subjectCondensed Matter
dc.titleSolution of the crystallographic phase problem by iterated projections
dc.typetext

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