2026-07-072026-07-07http://salesiana.dossiersoluciones.com/handle/123456789/156212We report on the magnetic properties of the layered perovskite PbVO(3). The results of magnetic susceptibility and specific heat measurements as well as band structure calculations consistently suggest that the S=1/2 square lattice of vanadium atoms in PbVO(3) is strongly frustrated due to next-nearest-neighbor antiferromagnetic interactions. The ratio of next-nearest-neighbor (J(2)) to nearest-neighbor (J(1)) exchange integrals is estimated to be J(2)/J(1)\approx 0.2-0.4. Thus, PbVO(3) is within or close to the critical region of the J(1)-J(2) frustrated square lattice. Supporting this, no sign of long-range magnetic ordering was found down to 1.8 K.4 pages, 4 figures, 2 tablesStrongly Correlated ElectronsMaterials ScienceFrustrated spin-1/2 square lattice in the layered perovskite PbVO(3)text