2026-07-072026-07-07http://salesiana.dossiersoluciones.com/handle/123456789/146848Single crystals of R$_2$CoGa$_8$ series of compounds were grown, for the first time, by high temperature solution growth (flux) method. These compounds crystallize in a tetragonal crystal structure with the space group $P4/mmm$. It has been found that R$_2$CoGa$_8$ phase forms only with the heavier rare earths, starting from Gd with a relatively large $c/a$ ratio of $\approx$ 2.6. The resultant anisotropic magnetic properties of the compounds were investigated along the two principal crystallographic directions of the crystal viz., along [100] and [001]. The nonmagnetic compounds Y$_2$CoGa$_8$ and Lu$_2$CoGa$_8$ show diamagnetic behavior down to the lowest temperature (1.8 K) pointing out the non-magnetic nature of Co in these compounds and a relatively low density of electronic states at the Fermi level. Compounds with the magnetic rare earths order antiferromagnetically at temperatures lower than 30 K. The easy axis of magnetization for R$_2$CoGa$_8$ (R = Tb, Dy and Ho) is found to be along the [001] direction and it changes to [100] direction for Er$_2$CoGa$_8$ and Tm$_2$CoGa$_8$. The magnetization behavior is analyzed on the basis of crystalline electric field (CEF) model. The estimated crystal field parameters explains the magnetocrystalline anisotropy in this series of compounds.In communication with prbStrongly Correlated Electronstext